It wasn’t clear when I first starting reading this post so just in case others stumble upon the same thing: this post is not about using U2F on the librem key itself. It’s how to configure a server or at least another machine to be authenticated with another U2F token, for example with a Yubikey.
As far as I know, the Librem Key still doesn’t support U2F, as discussed here:
Thanks for the tutorial by the way, it looks well made!